01Laser absorption spectroscopy and tomographic reconstruction
Using tunable laser absorption spectroscopy, we investigate spectral-line selection, signal analysis and quantitative temperature and species-concentration measurements for combustion environments. By arranging optical paths at different positions and viewing angles, we use tomography to reconstruct spatial distributions from line-integrated absorption signals. Particular attention is given to the effects of high-temperature spectroscopic models, flow-field nonuniformity, limited observations and measurement noise on reconstruction, improving spatial resolution and reliability in complex reacting flows.
02Diagnostics of multiphase reacting flows and flame dynamics
We use particle image velocimetry (PIV) to measure velocity fields and characterize recirculation, shear and turbulence structures. Phase Doppler particle analysis (PDPA) provides spray-droplet size and velocity measurements for studies of atomization, transport and gas–liquid interactions. Combined with reaction-zone imaging, these measurements reveal how fuel mixing, droplet evaporation and combustion influence one another, and clarify the relationships among flow fluctuations, vortical structures and flame response. Soot formation and transport are also included in our optical characterization of multiphase reacting flows.
03Imaging temperature and species-concentration fields
We combine laser absorption, laser-induced fluorescence (LIF), emission spectroscopy and infrared imaging to investigate multidimensional, time-resolved measurements of temperature and key species-concentration fields. For different species and measurement conditions, we establish quantitative relationships between optical signals and the quantities of interest by accounting for molecular excitation, collisional quenching and radiative transfer. Our focus is on the spatial distributions and transient evolution of reaction zones, localized high-temperature regions and combustion pollutants, providing experimental evidence for interactions among mixing, reactions and heat transfer.
04Advanced spectroscopy for reacting flows
We explore dispersion spectroscopy for combustion reacting flows, using gas-induced changes in optical phase to obtain information on species and thermodynamic states. This work examines the complementary roles of absorption and dispersion measurements and methods for extracting signals in complex environments. We also seek to explore broadband, high-resolution techniques such as optical frequency-comb and dual-comb spectroscopy for simultaneous multispecies measurements, analysis of overlapping spectra and diagnostics of transient reactions, extending the information available from conventional measurements using a small number of spectral lines.